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Reduction kinetics of SrFeO/CaO∙MnO nanocomposite as effective oxygen carrier for chemical looping partial

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 12,   Pages 1726-1734 doi: 10.1007/s11705-022-2188-5

Abstract: In this work, the kinetics of SrFeO<sub>3−<i>δi>sub>–CaO∙MnO nanocomposite reduction by methane wasof weight loss related to the partial oxidation is well fitted by the Avrami–Erofeyev equation with <i>ni> = 3 (A3 model) with an activation energy of 59.8 kJ∙mol‒1.rate law for the partial oxidation includes a solid conversion term whose expression is given by the A3

Keywords： chemical looping reforming     SrFeO<sub>3−<i>δi>sub>/CaO·MnO nanocomposite     reduction kinetics     Avrami–Erofeyev    

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g-CN-coated MnO hollow nanorod cathode for stable aqueous Zn-ion batteries

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 2,   Pages 217-225 doi: 10.1007/s11705-022-2214-7

Abstract: Herein, superior <i>αi>-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> was successfully prepared forstable zinc-ion batteries (ZIBs) cathode by introducing g-C<sub>3sub>N<sub>4sub> nanosheets.Compared with pure <i>αi>-MnO<sub>2sub>, <i>αi>-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> hasEven at 1 A·g–1, the <i>αi>-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub> still retains 100The <i>αi>-MnO<sub>2sub>@g-C<sub>3sub>N<sub>4sub>-based cathode has the highest energy density

Keywords： <i>αi>-MnO<sub>2sub> hollow nanorods     g-C<sub>3sub>N<sub>4sub>     heterojunction     aqueous Zn-ion    

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Denitrification performance and sulfur resistance mechanism of Sm–Mn catalyst for low temperature NH-SCR

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 5,   Pages 617-633 doi: 10.1007/s11705-022-2258-8

Abstract: MnO<sub><i>xi>sub> and Sm–Mn catalysts were prepared with the coprecipitation method, and they showedexcellent activities and sulfur resistances for the selective catalytic reduction of NO<sub><i>xi>sub> by NH<sub>3sub> between 50 and 300 °C in the presence of excess oxygen. 0.10Sm–Mn catalyst indicatedTherefore, it significantly enhances the NO conversion, N<sub>2sub> selectivity, and sulfur resistanceThe Bronsted acid sites strengthen significantly due to the addition of SO<sub>2sub>, enhancing the

Keywords： MnO<sub><i>xi>sub>     Sm–Mn     catalyst     NH<sub>3sub>-SCR     sulfur resistance    

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Evaluation of H<sub>2sub> on the Evolution Mechanism of NO<sub><i>xi>sub> Storage and Reductionover Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> Catalysts Article

Pan Wang, Jing Yi, Chuan Sun, Peng Luo, Lili Lei

Engineering 2019, Volume 5, Issue 3,   Pages 568-575 doi: 10.1016/j.eng.2019.02.005

Abstract:

In this investigation, Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> catalysts were preparedThe physical and chemical properties of the Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub>>xsub>, CeO<sub>2sub>, and BaCO<sub>3sub>, whose peaks were observed in X-ray diffraction(XRD) spectra, dispersed well on the γ-Al2O3, as shown by transmission electron microscope (TEMand conversion were increased when the time of H<sub>2sub> exposure (i.e., 30 s, 45 s, and 60 s) was

Keywords： Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> catalysts     Physicochemical properties     NO<sub><i>xi>sub> storageand reduction     NO<sub><i>xi>sub> emission     H<sub>2sub> reductant    

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Recent advances in special morphologic photocatalysts for NO removal

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 11, doi: 10.1007/s11783-022-1573-0

Abstract:

● Systematic information of recent progress in photocatalytic NO<sub> <i> x i>sub> removal is provided.

Keywords： NO<sub><i>xi>sub> removal     Photocatalyst     Graphene     C<sub>3sub>N<sub>4sub>     Bi-based compounds    

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Superior performance in visible-light-driven hydrogen evolution reaction of three-dimensionally ordered macroporous SrTiO decorated with ZnCdS

Frontiers of Chemical Science and Engineering 2021, Volume 15, Issue 6,   Pages 1561-1571 doi: 10.1007/s11705-021-2089-z

Abstract: In this study, we demonstrate the fabrication of three-dimensionally ordered macroporous SrTiO<sub>3sub> decorated with Zn<sub><i>xi>sub>Cd<sub>1−sub><sub><i>xi>sub>S nanoparticles for hydrogenapparent quantum efficiency of 35.9% at 420 nm, which is 4.2 and 23.9 times higher than those of pure Zn<sub>0.5sub>Cd<sub>0.5sub>S (4.67 mmol·g−1·h−1) and CdS (0.82 mmol·g−1

Keywords： three-dimensionally ordered macroporous SrTiO<sub>3sub>     Zn<sub><i>xi>sub>Cd<sub>1–sub><sub><i>xi>sub>S     visible light     hydrogen production     promotion mechanism    

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CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 5, doi: 10.1007/s11783-022-1539-2

Abstract:

• CeO<sub>2sub> doping significantly improved low-temperature NH<sub>3sub>-SCR activity on FeTiO<sub><i>xi>sub>.

Keywords： NH<sub>3sub>-SCR     CeO<sub>2sub> doping     Low-temperature NO<sub><i>xi>sub> removal     Improved redoxproperty     <i>In situi> XAFS analysis    

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Development of an H reduction and moderate oxidation method for 3,5-dimethylpyridine hydrogenation in

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 12,   Pages 1807-1817 doi: 10.1007/s11705-022-2243-2

Abstract: The Ru/C catalyst prepared by impregnation method was used for hydrogenation of 3,5-dimethylpyridineTherefore, an <i>in-situi> H<sub>2sub> reduction and moderate oxidation method was developed to increasethe highest 3,5-dimethylpyridine conversion was obtained for the Ru/C-i1 catalyst prepared by <i>in-situof the <i>in-situi> H<sub>2sub> reduction and moderate oxidized Ru/C-i2 catalyst, the interactionbetween RuO<sub><i>xi>sub> species and the support changed, and the hard-to-reduce RuO<sub><i>x<

Keywords： Ru/C catalyst     <i>in-situi> H<sub>2sub> reduction and moderate oxidation     <i>in-situi> reduction     non-<i>in-situi> reduction     hydrogenation of 3     5-dimethylpyridine    

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On the monolayer dispersion behavior of Co<sub>3sub>O<sub>4sub> on HZSM-5 support: designing applicable

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11,   Pages 1741-1754 doi: 10.1007/s11705-023-2332-x

Abstract: Based on monolayer dispersion theory, Co<sub>3sub>O<sub>4sub>/ZSM-5 catalysts with different loadingsCo<sub>3sub>O<sub>4sub> can spontaneously disperse on HZSM-5 support with a monolayer dispersionsites are crucial for the reaction, which can adsorb and activate NO<sub><i>xi>sub> and NH<sub>3Below the monolayer dispersion threshold, Co<sub>3sub>O<sub>4sub> is finely dispersed as sub-monolayerscapacity amount of Co<sub>3sub>O<sub>4sub> onto HZSM-5 support.

Keywords： Co<sub>3sub>O<sub>4sub>/ZSM-5     NO<sub><i>xi>sub>-SCR by NH<sub>3sub>     monolayer dispersionthreshold effect     surface acid sites     surface active O<sub>2sub>– anions    

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Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Frontiers of Environmental Science & Engineering 2017, Volume 11, Issue 6, doi: 10.1007/s11783-017-0976-9

Abstract: N O is a powerful greenhouse gas and plays an important role in destructing the ozone layer. This present work investigated the effects of Pd doping on N O formation over Pt/BaO/Al O catalyst. Three types of catalysts, Pt/BaO/Al O , Pt/Pd mechanical mixing catalyst (Pt/BaO/Al O +Pd/Al O ) and Pt-Pd co-impregnation catalyst (Pt-Pd/BaO/Al O ) were prepared by incipient wetness impregnation method. These catalysts were first evaluated in NSR activity tests using H /CO as reductants and then carefully characterized by BET, CO chemisorption, CO-DRIFTs and H -TPR techniques. In addition, temperature programmed reactions of NO with H /CO were conducted to obtain further information about N O formation mechanism. Compared with Pt/BaO/Al O , (Pt/BaO/Al O +Pd/Al O ) produced less N O and more NH during NO storage and reduction process, while an opposite trend was found over (Pt-Pd/BaO/Al O +Al O ). Temperature programmed reactions of NO with H /CO results showed that Pd/Al O component in (Pt/BaO/Al O +Pd/Al O ) played an important role in NO reduction to NH , and the formed NH could reduce NO to N leading to a decrease in N O formation. Most of N O formed over (Pt-Pd/BaO/Al O +Al O ) was originated from Pd/BaO/Al O component. H -TPR results indicated Pd-Ba interaction resulted in more difficult-to-reduce PdO species over Pd/BaO/Al O , which inhibits the NO dissociation and thus drives the selectivity to N O in NO reduction.

Keywords： NO<sub><i>xi>sub> storage reduction     Pt/BaO/Al<sub>2sub>O<sub>3sub>     Pd doping     N<sub>2sub>O formation    

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NiFeRuO<sub><i>xi>sub> nanosheets on Ni foam as an electrocatalyst for efficient

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11,   Pages 1698-1706 doi: 10.1007/s11705-023-2334-8

Abstract: The electrocatalyst NiFeRuO<sub><i>xi>sub>/NF, comprised of NiFeRuO<sub><i>xi>sub> nanosheetsNiFeRuO<sub><i>xi>sub>/NF displays high electrocatalytic activity and stability for overall alkalineA solar-driven system containing such a bifunctional NiFeRuO<sub><i>xi>sub>/NF has an almost 100%The NiFeRuO<sub><i>xi>sub> coating around Ni foam is an anti-corrosion layer and also a critical

Keywords： NiFeRuO<sub><i>xi>sub> nanosheets     Ni foam     electrocatalysis     overall seawater splitting     solar-driven    

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NO<sub><i>xi>sub> and H<sub>2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

Frontiers in Energy 2021, Volume 15, Issue 1,   Pages 4-13 doi: 10.1007/s11708-020-0804-y

Abstract: Low NO combustion of blended coals is widely used in coal-fired boilers in China to control NO emission; thus, it is necessary to understand the formation mechanism of NO and H S during the combustion of blended coals. This paper focused on the investigation of reductive gases in the formation of NO and H S in the reductive zone of blended coals during combustion. Experiments with Zhundong (ZD) and Commercial (GE) coal and their blends with different mixing ratios were conducted in a drop tube furnace at 1200°C–1400°C with an excessive air ratio of 0.6–1.2. The coal conversion and formation characteristics of CO, H S, and NO in the fuel-rich zone were carefully studied under different experimental conditions for different blend ratios. Blending ZD into GE was found to increase not only the coal conversion but also the concentrations of CO and H S as NO reduction accelerated. Both the CO and H S concentrations inblended coal combustion increase with an increase in the combustion temperature and a decrease in the excessive air ratio. Based on accumulated experimental data, one interesting finding was that NO and H S from blended coal combustion were almost directly dependent on the CO concentration, and the CO concentration of the blended coal combustion depended on the single char gasification conversion.Thus, CO, NO , and H S formation characteristics from blended coal combustion can be well predicted by single char gasification kinetics.

Keywords： blended coal combustion     NO<sub><i>x i>sub>formation     H<sub>2sub>S formation     air staged combustion    

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Thermal and Mechanical Properties Optimization of <i>ABi>O<sub>4sub> Type EuNbO<sub>4sub> By the<i>Bi>-Site Substitution of Ta Article

Lin Chen, Jing Feng

Engineering 2020, Volume 6, Issue 2,   Pages 177-184 doi: 10.1016/j.eng.2019.12.006

Abstract:

Ferroelastic ABO<sub>4sub> type RETaO<sub>4sub> and RENbO<sub>4sub> ceramics (where>4sub> have been found to be better than those of RENbO<sub>4sub>.>4sub> fabricated through a solid-state reaction (SSR).The Young's modulus and the thermal expansion coefficient (TEC) of EuNbO<sub>4sub> are effectivelyThe results indicate that the thermal and mechanical properties of EuNbO<sub>4sub> can be effectually

Keywords： Thermal barrier coatings     Rare earth niobates     Substitution     Thermal conductivity     Thermal expansion coefficients     Young’s modulus    

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Band-gap tunable (Ga<i><sub>xsub>i>In<sub>1−sub><i><sub>xsub>i>)<sub>2sub>O<sub>3sub> layer Research Articles

Fabi Zhang, Jinyu Sun, Haiou Li, Juan Zhou, Rong Wang, Tangyou Sun, Tao Fu, Gongli Xiao, Qi Li, Xingpeng Liu, Xiuyun Zhang, Daoyou Guo, Xianghu Wang, Zujun Qin,zhangfabi@outlook.com,qinzj@guet.edu.cn

Frontiers of Information Technology & Electronic Engineering 2021, Volume 22, Issue 10,   Pages 1370-1378 doi: 10.1631/FITEE.2000330

Abstract: Multicomponent oxide (GaIn)O films are prepared on (0001) sapphire substrates to realize a tunable band-gap by technology followed by thermal annealing. The optical properties and band structure evolution over the whole range of compositions in ternary compounds (GaIn)O are investigated in detail. The X-ray diffraction spectra clearly indicate that (GaIn)O films with Ga content varying from 0.11 to 0.55 have both cubic and monoclinic structures, and that for films with Ga content higher than 0.74, only the monoclinic structure appears. The transmittance of all films is greater than 86% in the visible range with sharp absorption edges and clear fringes. In addition, a blue shift of ultraviolet absorption edges from 380 to 250 nm is noted with increasing Ga content, indicating increasing band-gap energy from 3.61 to 4.64 eV. The experimental results lay a foundation for the application of transparent conductive compound (GaIn)O thin films in photoelectric and photovoltaic industry, especially in display, light-emitting diode, and solar cell applications.

Keywords： (GaxIn1−x)2O3薄膜；带隙可调谐；磁控溅射    

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Atmospheric heterogeneous reaction of chlorobenzene on mineral -FeO particulates: a chamber experiment study

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 11, doi: 10.1007/s11783-023-1734-9

Abstract:

● Photochemical conversion of chlorobenzene (CB) on α-Fe<sub>2sub>O<sub>3sub> was evaluated.

Keywords： Photochemical conversion     Chlorobenzene     <i>αi>-Fe<sub>2sub>O<sub>3sub>     PCDD/Fs     Mineral particulate    

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Title Author Date Type Operation

Reduction kinetics of SrFeO/CaO∙MnO nanocomposite as effective oxygen carrier for chemical looping partial

Journal Article

g-CN-coated MnO hollow nanorod cathode for stable aqueous Zn-ion batteries

Journal Article

Denitrification performance and sulfur resistance mechanism of Sm–Mn catalyst for low temperature NH-SCR

Journal Article

Evaluation of H<sub>2sub> on the Evolution Mechanism of NO<sub><i>xi>sub> Storage and Reductionover Pt–Ba–Ce/γ-Al<sub>2sub>O<sub>3sub> Catalysts

Pan Wang, Jing Yi, Chuan Sun, Peng Luo, Lili Lei

Journal Article

Recent advances in special morphologic photocatalysts for NO removal

Journal Article

Superior performance in visible-light-driven hydrogen evolution reaction of three-dimensionally ordered macroporous SrTiO decorated with ZnCdS

Journal Article

CeO doping boosted low-temperature NH-SCR activity of FeTiO catalyst: A microstructure analysis and reaction mechanistic study

Journal Article

Development of an H reduction and moderate oxidation method for 3,5-dimethylpyridine hydrogenation in

Journal Article

On the monolayer dispersion behavior of Co<sub>3sub>O<sub>4sub> on HZSM-5 support: designing applicable

Journal Article

Effects of Pd doping on N

Mingxin Dong, Jun Wang, Jinxin Zhu, Jianqiang Wang, Wulin Wang, Meiqing Shen

Journal Article

NiFeRuO<sub><i>xi>sub> nanosheets on Ni foam as an electrocatalyst for efficient

Journal Article

NO<sub><i>xi>sub> and H<sub>2sub>S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

Journal Article

Thermal and Mechanical Properties Optimization of <i>ABi>O<sub>4sub> Type EuNbO<sub>4sub> By the<i>Bi>-Site Substitution of Ta

Lin Chen, Jing Feng

Journal Article

Band-gap tunable (Ga<i><sub>xsub>i>In<sub>1−sub><i><sub>xsub>i>)<sub>2sub>O<sub>3sub> layer

Fabi Zhang, Jinyu Sun, Haiou Li, Juan Zhou, Rong Wang, Tangyou Sun, Tao Fu, Gongli Xiao, Qi Li, Xingpeng Liu, Xiuyun Zhang, Daoyou Guo, Xianghu Wang, Zujun Qin,zhangfabi@outlook.com,qinzj@guet.edu.cn

Journal Article

Atmospheric heterogeneous reaction of chlorobenzene on mineral -FeO particulates: a chamber experiment study

Journal Article